Beyond the single-atom response in absorption line shapes: probing a dense, laser-dressed helium gas with attosecond pulse trains.
نویسندگان
چکیده
We investigate the absorption line shapes of laser-dressed atoms beyond the single-atom response, by using extreme ultraviolet (XUV) attosecond pulse trains to probe an optically thick helium target under the influence of a strong infrared (IR) field. We study the interplay between the IR-induced phase shift of the microscopic time-dependent dipole moment and the resonant-propagation-induced reshaping of the macroscopic XUV pulse. Our experimental and theoretical results show that as the optical depth increases, this interplay leads initially to a broadening of the IR-modified line shape, and subsequently, to the appearance of new, narrow features in the absorption line.
منابع مشابه
Absorption and emission of single attosecond light pulses in an autoionizing gaseous medium dressed by a time-delayed control field
An extreme ultraviolet (EUV) single attosecond pulse passing through a laser-dressed dense gas is studied theoretically. The weak EUV pulse pumps the helium gas from the ground state to the 2s2p(1P ) autoionizing state, which is coupled to the 2s2(1S) autoionizing state by a femtosecond infrared laser with the intensity in the order of 1012 W/cm2. The simulation shows how the transient absorpti...
متن کاملAttosecond-resolved evolution of a laser-dressed helium atom: interfering excitation paths and quantum phases.
Using high-order harmonic attosecond pulse trains, we investigate the photoionization dynamics and transient electronic structure of a helium atom in the presence of moderately strong (∼10(12) W cm(-2)) femtosecond laser pulses. We observe quantum interferences between photoexcitation paths from the ground state to different laser-dressed Floquet state components. As the intensity ramps on fem...
متن کاملAttosecond probing of instantaneous ac Stark shifts in helium atoms
Based on the numerical solutions of the time-dependent Schrödinger equation within the single-active-electron approximation, we propose a method for observing instantaneous atomic level shifts in an oscillating strong infrared (IR) field with sub-IR-cycle time resolution, by using a single tunable attosecond (SA) pulse to probe excited states of the perturbed atom. The ionization probability in...
متن کاملXUV Transient Absorption Spectroscopy: Probing Laser-Perturbed Dipole Polarization in Single Atom, Macroscopic, and Molecular Regimes
We employ an extreme ultraviolet (XUV) pulse to impulsively excite dipole polarization in atoms or molecules, which corresponds to coherently prepared superposition of excited states. A delayed near infrared (NIR) pulse then perturbs the fast evolving polarization, and the resultant absorbance change is monitored in dilute helium, dense helium, and sulfur hexafluoride (SF6) molecules. We observ...
متن کاملPhotoabsorption of attosecond XUV light pulses by two strongly laser-coupled autoionizing states
We study theoretically the photoabsorption spectra of an attosecond extreme ultraviolet (XUV) pulse by a laser-dressed atomic system. A weak XUV excites an autoionizing state which is strongly coupled to another autoionizing state by a laser. The theory was applied to explain two recent experiments [Loh, Greene, and Leone, Chem. Phys. 350, 7 (2008); Wang, Chini, Chen, Zhang, Cheng, He, Cheng, W...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید
ثبت ناماگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید
ورودعنوان ژورنال:
- Physical review letters
دوره 114 14 شماره
صفحات -
تاریخ انتشار 2015